I know it may sound silly, but love can make people do some pretty crazy (and even straight up evil) things so is there a god/demon lord/whatever of love who's evil?
Archdevil Belial, The Pale Kiss - adultery, desire
Daemon harbinger Slandrais, The Watcher In The Walls - leechery, love potions and obsessions.
Daemon harbinger Laivatiniel, The Chains And The Cradle - unhealthy parental love and coddling.
Daemon harbinger Folca, The Gaunt Stranger - abductions (including those motivated by love)
Demon lord Nocticula, Our Lady In Shadow, The First Succubus - lust, seduction, carnal attraction
Demon lord Socothbenoth, The Silken Sin - perversion, deviants, leecherous maniacs
Eldest The Green Mother, The Feasting Flower - seduction (and intrigue)
Infernal Duke Zepar, The Forever Sire - abduction, rape
Nascent Demon Lord Shamira, Princess Of The Porphyry City - seduction of the pure
Oni Daimyo Onmyuza, Dancer in Flesh - orgies
Orc deity Verex, The Despoiler - rape (and pillaging)
You also have the minor goddess Naderi, the Lost Maiden; she's neutral, but she patrons forbidden relationships and love-motivated suicides.
Love subdomain (will have to scroll down)
The only one of note that Adjoint didn't mention is Ardad Lili, a minor deity from Hell.
Calistria has Evil worshippers.
Calistria in general?
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Dispater is an Archdevil who believes in courtly love, and has even married on multiple occasions. His current wife is Erecura, a deity of divination and his closest adviser. He is the father of Ragathiel by his previous wife, Feronia, with whom he is still on friendly terms. If you're looking for an Evil deity who would approve of romance and love, Dispater is likely your best choice.